Publication

Advanced Multifunctional Nanocomposite Lab

Selected Representative Publications

  • 2023
  • Giant thermal rectification efficiency by geometrically enhanced asymmetric non-linear radiation
  • Seongkyun Kim , Taeyeop Kim , Jaehyun Sung , Yongjun Kim , Dongwoo Lee and Seunghyun Baik Materials Horizons
  • Thermal rectification is an asymmetric heat transport phenomenon where thermal conductance changes depending on the temperature gradient direction. The experimentally reported efficiency of thermal rectification materials and devices, which are applicable for a wide range of temperatures, is relatively low. Here we report a giant thermal rectification efficiency of 218% by maximizing asymmetry in …
  • 2022
  • Invariable resistance of conductive nanocomposite over 30% strain
  • C. MUHAMMED AJMAL, SEOKJAE CHA, WONJOON KIM, K. P. FASEELA, HEEJUN YANG, AND SEUNGHYUN BAIK Science Advances
  • The dependence of the electrical resistance on materials’ geometry determines the performance of conductive nanocomposites. Here, we report the invariable resistance of a conductive nanocomposite over 30% strain. This is enabled by the in situ–generated hierarchically structured silver nanosatellite particles, realizing a short interparticle distance (4.37 nm) in a stretchable silicone rubber matr…
Simple and efficient synthesis of nanograin structured single phase filled skutterudite for high thermoelectric performance
Author
Sanghoon Lee, Kyu Hyoung Lee, Young-Min Kim, Hyun Sik Kim, G. Jeffrey Snyder, Seunghyun Baik, Sung Wng Kim
Journal
Acta Materialia
Vol
142
Page
8-17
Year
2018
Filled skutterudites are promising mid-to-high temperature range thermoelectric materials for power generation, however, a traditional melt-solidification process followed by annealing (TMA) and powder metallurgical sintering requires a long processing time more than 10 days to ensure the structural and compositional homogeniety of materials with a high thermoelectric conversion efficiency zT. To address this, we herein report a simple and efficient synthesis of high-performance n- and p-type filled skutterudites that successfully produces a complete single phase from single to multiple filled materials in a day. The nanograin (∼440 nm) structured bulks are prepared from the combined process of temperature-regulated melt spinning (MS) using ingots and short-time spark plasma sintering (SPS). The controlled phase evolution and transformation by adjusting rapid solidification and densification conditions are demonstrated by a comprehensive analysis including structure refinement and atomic-scale observation, verifying the desired occupancy and random distribution of filling elements, respectively. The maximum zT values of filled skutterudites fabricated here were 1.48 ± 0.17 at 800 K for n-type In0.12Yb0.20Co4.00Sb11.84 and 1.15 ± 0.13 at 750 K for p-type Ce0.91Fe3.40Co0.59Sb12.14, which are comparable to the highest zT values reported for filled skutterudites fabricated by TMA-based processes. Superior reproducibility achieved in shortened processing time enables the present synthetic process to be utilized for commercial manufacturing process that can be readily applied to massive production of bulk filled skutterudites for high-performance thermoelectric power generators.